• Zachary Levi is Chuck, a geeky computer expert who works at Buy More. Zachary Levi was Kipp Steadman in Less Than Perfect.
• Adam Baldwin is Major John Casey, who works for the NSA and is in charge of protecting Chuck. Adam was Jayne Cobb on Firefly and Chad Shelten on Day Break, among many other roles.
• Yvonne Strzechowski is top CIA agent Sarah Walker, who becomes Chuck's partner.
• Joshua Gomez as Morgan, Chuck's best friend. Joshua was James Mackeroy on Without a Trace and Scott on Invasion.
• Sarah Lancaster as Ellie, Chuck's sister. Sarah did a short but memorable stint as Lisa the Gift Shop Girl on Scrubs, and was Madison on Everwood.
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